Journal Article

·2021

Determination of selenite and selenomethionine in kefir grains by reversed‐phase high‐performance liquid chromatography–inductively coupled plasma‐optical emission spectrometry

Süleyman Bodur YTU , Miray Öner YTU , Sezin Erarpat YTU , Sezgin Bakırdere YTU

Journal of Separation Science

Abstract

Abstract A new and efficient reversed‐phase high‐performance liquid chromatography–inductively coupled plasma–optical emission spectrometry method was developed for the simultaneous separation and determination of SeO 3 2– and seleno‐ dl ‐methionine in kefir grains. For the system, limits of detection and quantitation values for SeO 3 2– and seleno‐ dl ‐methionine were calculated as 0.52/1.73 mg/kg (as Se) and 0.26/0.87 mg/kg (as Se), respectively. After performing the system analytical performance, recovery experiment was done for kefir grains and percent recovery results for SeO 3 2– and seleno‐ dl ‐methionine were calculated as 98.4 ± 0.8% and 93.6 ± 1.0%, respectively. It followed by the feeding studies that the kefir grains were exposed to three different concentrations of SeO 3 2– (20, 30, and 50 mg/kg) for approximately 4 days at room temperature to investigate the conversion/non‐conversion of SeO 3 2– to seleno‐ dl ‐methionine. Next, the fed grains were extracted with tetramethylammonium hydroxide pentahydrate solution (20%, w/w) and then sent to the developed system. There was no detectable seleno‐ dl ‐methionine found in fed kefir grains at different concentrations of SeO 3 2– while inorganic or elemental selenium in the fed kefir grains was determined between 1579.5 – 3116.0 mg/kg (as Se). Selenium species in the kefir grains samples was found in the form of SeO 3 2– proved by using an anion exchange column.

Keywords

Selenium Chemistry Inductively coupled plasma Chromatography High-performance liquid chromatography Detection limit Analytical Chemistry (journal) Inductively coupled plasma mass spectrometry Ion chromatography Mass spectrometry Plasma

Subject Areas

Selenium in Biological Systems ·Nutrition and Dietetics ·Health Sciences
Mercury impact and mitigation studies ·Health, Toxicology and Mutagenesis ·Physical Sciences
Trace Elements in Health ·Nutrition and Dietetics ·Health Sciences

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