Abstract
The dimensionality-driven two-photon absorption (2PA) enhancement effect is investigated in a series of functionalized bipyridyl Ru-complexes. Our design strategy leads to very high 2PA responses up to ∼1500 GM. However, we highlight that the 2PA performance vs. dimensionality correlation reaches an unexpected limit stemming from 'anti-cooperative' interchromophoric couplings.
Keywords
Curse of dimensionality
Series (stratigraphy)
Absorption (acoustics)
Ruthenium
Two-photon absorption
Photochemistry
Photon
Chemistry
Chemical physics
Physics
Computer science
Optics
Catalysis
Organic chemistry
Laser
Subject Areas
Nonlinear Optical Materials Studies
·Biomedical Engineering ·Physical Sciences
Porphyrin and Phthalocyanine Chemistry
·Materials Chemistry ·Physical Sciences
Photochromic and Fluorescence Chemistry
·Materials Chemistry ·Physical Sciences
Citations by Year
2021: 2
2022: 3
2023: 1
2024: 1
2025: 2
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